Correspondents include C. D. Ebeling, Alexander von Humboldt, and Henry Melchior Muhlenberg.

This set of journals, copied legibly but with many excisions into the last volume, 914 Sm61, is from a tour of Germany, Denmark, Sweden, France, and England, to inspect technological improvements in manufacturing and mining. There are accounts of visits with C.D. Ebeling, Friedrich Klopstock, J.A.J. Reimarus, Anders Sparmann, and Karl P. Thunberg. Smith bequeathed this journal to the American Philosophical Society with the request that it be published if found to contain information "useful to the manufactories of my country."